Not necessarily villains, but definitely jerks.
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Peter Pan was an arse in Kingdom Hearts.
I really just want to kill this guy. I seriously was excited when Sin attacked Luca at first, I thought it might have killed him and the other Goers. But especially him.
The Reapers are coming to wipe out all life, continuing an endless spiral of extermination. Saren finds out in advance. What does he do? He decides that it's a better bet to throw in with the merciless killing machines rather than warn anyone. What an arse.
Governor Jerk-Face here is a complete butt crack.
Seymour is a jerk whose impossible hairstyle was under my skin long before his glowing personality came to light and he began making advances on Yuna and such, much less the nihilism.
Charming to the last, Magashi shows his love for humanity, and amazing devotion to the greater good time and time again. His is an example of heroic proportions for all to follow. If you couldn't tell, I am being extremely sarcastic.