Devil May Cry 3 -- because it's a great game, challenging (though definitely beatable) and also has enough interesting and outlandish cutscenes, which make it a fun game to watch.
Persona 3 -- which requires no explanation, I think.
Condemned I and II -- excellent games, which are fun to play and feature plenty of brutality to keep things interesting.
The Yakuza games -- they're all worth playing, honestly.
Telltale games -- The Walking Dead, the Game of Thrones game: they would be interesting to watch and allow for group-based decision-making, just like Persona 4 did at the time (which made it perfect for an Endurance Run) or, more recentl, Until Dawn.
The Witcher 1 or The Witcher 2 -- requires little explanation, I think.
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