He would be so challenging to create in Nolan's realistic paradigm, but man, would he be fascinating!
I'm all for Mr. Freeze at this point - recent iterations have fleshed out a beautifully tragic character. (Animated Series, Heart of Ice. will blow. your. mind.)
The filmmakers would have a huge task of recreating the Freeze/Fries in a more grounded context- make his methods more feasible, whilst maintaining the concept - see Scarecrow in 'Begins.
I see Stellan Skarsgaard. He has such a grim, sad face, and his European heritage couldn't hurt.
Hulk, I absolutely love the Knightfall idea - the story arc seems perfectly suited to Nolan's believable Gotham. Azrael's violence and lack of mortal restraint would create such a great contast to the ideas so starkly analyzed in the Dark Knight - how far is one willing to go to do the "right thing?"
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